Mapping Catalyst–Solvent Interplay in Competing Carboamination/Cyclopropanation Reactions
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Selectivity and activity maps can be used to predict and rationalize reaction outcomes based on catalyst and solvent choice. Here, there utility is demonstrated by examining competing carboamination/cyclopropanation reactions catalyzed by Group 9 catalysts featuring cyclopentadienyl ligands, which reveals an interesting energetic interplay involving the role of the solvent and of the catalyst.
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2023-06-12
