Data underlying the publication: Beneficial redox activity of halide solid electrolytes empowering high-performance anodes in all-solid-state batteries

This directory contains raw data (of main figure 1-6 in manuscript) that enables to reproduce the analysis done in: "Beneficial redox activity of halide solid electrolytes empowering high-performance anodes in all-solid-state batteries" by Zhu Cheng, Wenxuan Zhao, Qidi Wang, Chenglong Zhao, Anastasia K. Lavrinenko, Alexandros Vasileiadis, Victor Landgraf, Lars Bannenberg, Yuhang Li, Junwei Liang, Ming Liu, Swapna Ganapathy and Marnix Wagemaker. This directory contains: cyclic voltammetry data, electrochemical cycling data, NMR and XRD data of LYCB-CNF demonstrating the reversible redox behavior of LYCB as presented in Figure 1 in the manuscript; Convex hull calculation and RDF data obtained for LixYCl3Br3 through AIMD simulations as presented in Figure 2 in the manuscript; Evolution of the Li-ion kinetics of LYCB during discharge-charge from EIS and their corresponding DRT analysis demonstrating the improved Li-ion conductivity of LYCB after lithiation as presented in Figure 3 in the manuscript; Electrochemical, EIS, XPS and NMR characterization of the LYCB-based RP anode and LPSC-based RP anode demonstrating the superior compatibility of LYCB over LPSC as presented in Figure 4 in the manuscript; Electrochemical performance of the Li-In|LYCB|RP-LYCB half-cell and the LCO-LYCB and NMC-LYCB|LYCB|RP-LYCB full-cells as presented in Figure 5 in the manuscript; Electrochemical cycling and XRD data of the LZC-CNF mixture demonstrating the generality of the beneficial redox activity in trigonal LZC as presented in Figure 6 in the manuscript.<br>

本数据集目录包含论文手稿中图1至图6的原始实验数据，可复现朱诚（Zhu Cheng）、赵文轩（Wenxuan Zhao）、王启迪（Qidi Wang）、赵成龙（Chenglong Zhao）、阿纳斯塔西娅·K·拉夫连科（Anastasia K. Lavrinenko）、亚历山德罗斯·瓦西利亚迪斯（Alexandros Vasileiadis）、维克多·兰德里格拉夫（Victor Landgraf）、拉斯·班嫩贝格（Lars Bannenberg）、李宇航（Yuhang Li）、梁俊伟（Junwei Liang）、刘明（Ming Liu）、斯瓦普娜·加纳帕蒂（Swapna Ganapathy）与马尔尼克斯·瓦格马凯尔（Marnix Wagemaker）发表的论文《卤化物固态电解质的有益氧化还原活性助力全固态电池高性能负极》"Beneficial redox activity of halide solid electrolytes empowering high-performance anodes in all-solid-state batteries"中的分析结果。本目录包含以下内容：用于验证手稿中图1所示LYCB可逆氧化还原行为的LYCB-CNF材料的循环伏安法数据、电化学循环数据、核磁共振（Nuclear Magnetic Resonance, NMR）与X射线衍射（X-ray Diffraction, XRD）数据；通过从头算分子动力学（Ab Initio Molecular Dynamics, AIMD）模拟得到的LixYCl3Br3的凸包计算数据与径向分布函数（Radial Distribution Function, RDF）数据，对应手稿中图2的内容；通过电化学阻抗谱（Electrochemical Impedance Spectroscopy, EIS）得到的LYCB在充放电过程中的锂离子动力学演化数据及其对应的分布弛豫时间（Distribution of Relaxation Times, DRT）分析结果，用以证明锂化后LYCB的锂离子电导率得到提升，对应手稿中图3的内容；基于LYCB的RP负极与基于LPSC的RP负极的电化学表征、EIS、X射线光电子能谱（X-ray Photoelectron Spectroscopy, XPS）与NMR表征数据，用以证明LYCB相较于LPSC具有更优异的兼容性，对应手稿中图4的内容；Li-In|LYCB|RP-LYCB半电池以及锂钴氧化物（Lithium Cobalt Oxide, LCO）-LYCB与镍锰钴三元材料（Nickel Manganese Cobalt, NMC）-LYCB|LYCB|RP-LYCB全电池的电化学性能数据，对应手稿中图5的内容；LZC-CNF混合物的电化学循环数据与XRD数据，用以验证三方相LZC中有益氧化还原活性的普适性，对应手稿中图6的内容。