Study of the Stochastic Nature of Nucleation in Freeze-Drying

The hypothesis of this article is to investigate the stochastic nature of nucleation, with a primary focus o analyzing the order of nucleation events and the nucleation temperature. the study aims to determine to what extent fluctuations influence the nucleation process under controlled conditions.
in this work, we analyze the impact of various factors - such as temperature history, system size, and others control parameters. we assess the variability of nucleation behavior and distinguish between randomfluctuations and systematic trends.