Atmospheric Halocarbon Observations at Beromünster, Switzerland, and Bayesian Inverse Modeling to assess Emissions

Atmospheric halocarbon (CFCs, halons, HCFCs, HFCs, PFCs, SF6, NF3, HFOs) and carbon monoxide (CO) observations (mole fractions) from the tall tower site at Beromünster, Switzerland (47.2 °N, 8.2 °E, 797 m a.s.l., 212 m a.g.l.), covering the period September 2019 to September 2020. The halocarbon measurements were conducted using a Medusa pre-concentration unit, coupled to gas chromatography (Agilent 6890N) and mass spectrometry (Agilent 5975, GC-MS).

For further details see: Miller, B. R., Weiss, R. F., Salameh, P. K., Tanhua, T., Greally, B. R., Mühle, J., and Simmonds, P. G.: Medusa: A Sample Preconcentration and GC/MS Detector System for in Situ Measurements of Atmospheric Trace Halocarbons, Hydrocarbons, and Sulfur Compounds, Anal. Chem., 80, 1536–1545, https://doi.org/10.1021/ac702084k, 2008).

The data format follows that used within the AGAGE network (see AGAGE data archive: http://agage.mit.edu/data/agage-data).

Data results for the Bayesian inversion conducted based on the measurement data from Beromünster to assess Swiss halocarbon emissions. Files are provided in netCDF format for the 28 individual substances discussed in (Rust, D. et al., 2022, Swiss halocarbon emissions for 2019 to 2020 assessed from regional atmospheric observations, Atmospheric Chemistry and Physics). Each file contains the a priori and a posteriori emissions as used or calculated in the Bayesian inversion. Data are provided on the grid used in the inversion (irregular longitude/latitude). Metadata are included as netCDF attributes. The netCDF files follow the CF conventions and are readable with any netcdf interface/tool.