Dataset for 'Anisotropic Phonon Dynamics and Transport Properties in Actinide van der Waals Semiconductor USe3'

This dataset contains raw and processed data supporting the study 'Probing Anisotropic Phonon Dynamics and Transport Properties in Uranium-Based 2D Semiconductors.' The data include DFT input/output files (VASP, Phonopy, ShengBTE), raw Raman and strain-dependent spectra, transport and magnetization measurement data, and microscopy characterization (SEM, TEM, EDS, XRD). The dataset underpins the findings described in the publication, detailing the anisotropic electronic, phononic, and transport behavior of USe₃ as a van der Waals actinide analogue of transition metal trichalcogenides.