Quantum chemical sensing using molecular triplet qubits in a flexible metal–organic framework
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Fig. 2. b, Plot of T2 obtained by the single-exponential fitting of the spin echo decay curves
against the unit cell volume of MIL-53. c, Spin echo decay curves after pulsed
photoexcitation at 532 nm for empty (D-MIL-53⸧DAT) and guest-filled (D-MIL-
53⸧[DAT+guest]) samples at room temperature.
Fig. 3. a, Time-resolved
EPR spectra at 0.1–0.5 μs for empty (D-MIL-53⸧DAT) and guest-filled (D-MIL-
53⸧[DAT+guest]) samples at room temperature. b, Decays of the ESR peaks at higher and lower magnetic field after pulsed
photoexcitation at 532 nm for empty (D-MIL-53⸧DAT) and guest-filled (D-MIL-
53⸧[DAT+guest]) samples at room temperature.
Fig. 4. Dependence of T2 on volume fraction occupied by the guest.
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创建时间：
2024-09-05
