Imaging the state-to-state charge-transfer dynamics between the spin-orbit excited Ar<sup>+</sup>(<sup>2</sup>P<sub>1/2</sub>) ion and N<sub>2</sub>
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The data reported a synergistic experimental and theoretical investigation on the charge-transfer dynamics between the spin-orbit excited Ar+(2P1/2) and N2, which has been rarely studied before. The product vibrational, rotational, and angular distributions are partially resolved by the high-resolution three-dimensional VMI imaging. Qualitatively, the trajectory surface-hopping calculations reproduced several main features of the experimental observations.
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2024-02-03
