Catalytic Asymmetric Stetter Reaction Onto Vinylphosphine Oxides and Vinylphosphonates
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An intramolecular Stetter reaction of vinylphosphine oxides and vinylphosphonates has been developed. Treatment of an aldehyde with a nucleophilic N-heterocyclic carbene catalyst allows for addition of an acyl anion equivalent into a vinylphosphine oxide or vinylphosphonate Michael acceptor in yields up to 99% and ee values up to 96%.
创建时间：
2008-07-17
