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Local Atom Disorder Mediated Crystal Facet Valence State of PtCu Alloy for Ultrafast Ammonia Oxidation Dehydrogenation

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科学数据银行2025-04-21 更新2026-04-23 收录
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https://www.scidb.cn/detail?dataSetId=4f10bac75f1c417b8b1db4622c5f7008
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资源简介:
Pt (200) facet of platinum-based alloys exhibit high potential in ammonia oxidation reaction (AOR), but is still a huge bottleneck in activity enhancement due to the sluggish NHx-dehydrogenation kinetics and H-poisoning. Herein, a novelly local-disordered PtCu alloy, with an increasing low-valence-platinum ratio on the (200) facet by H2/Ar post-annealing ambient, was engineered to atomically boost AOR dehydrogenation behaviour through the reconstruction microenvironment of Pt (200) plane.
提供机构:
Jianan Su
创建时间:
2025-04-15
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