Stereoselective Synthesis of Highly Substituted Δ-Pyrrolines: <i>exo</i>-Selective 1,3-Dipolar Cycloaddition Reactions with Azlactones
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We report herein a silver(I)-catalyzed exo-selective synthesis of highly substituted Δ1-pyrroline scaffolds from amino acid-derived münchnones. Silver acetate successfully catalyzed the cycloaddition reaction of azlactones with alkenes, generating Δ1-pyrrolines in very good yields without isomerization to the Δ-pyrrolines or decarboxylation.
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2004-10-13
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