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Data Underpinning: Disordered ground state in the 3D face-centred frustrated spin-5/2 system MnSn(OH)₆

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DataCite Commons2025-07-22 更新2025-04-16 收录
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https://opara.zih.tu-dresden.de/items/1f5e25da-16c4-4cae-a362-cf838b586d79
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This contains the data underpinning our paper on MnSn(OH)₆. The abstract of the article is reproduced below: Frustrated magnetism in face-centered cubic (fcc) magnetic sublattices remains underexplored but holds considerable potential for exotic magnetic behavior. Here, we report on the crystal structural, magnetic and thermodynamic properties of the A-site-vacant double hydroxide perovskite MnSn(OH)₆. Despite dominant antiferromagnetic interactions among Mn²⁺ moments, evidenced by a negative Curie-Weiss temperature, the lack of a sharp thermodynamic transition down to 350 mK implies the absence of long-range magnetic order. However, a broad hump at 1.6 K suggests short-range correlations and spin freezing, with power-law behavior consistent with a spin-glass state. Neutron diffraction at low temperatures confirms the presence of three-dimensional (3D) antiferromagnetic correlations, manifesting as diffuse magnetic scattering with a correlation length ξ = 24.66 Å and a magnetic propagation vector k = (0 0 ½) at 20 mK.
提供机构:
Technische Universität Dresden
创建时间:
2025-03-06
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