POPE monthly emissions for ICON-ART PRIEST v1.0
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This dataset provides monthly gridded atmospheric emissions for two PFCAs (PFOA and PFNA) and their precursor compounds (8:2-FTOH, 8:2-FTO, and 8:2-FTI) covering 1950 – 2019. It is derived from the annual 0.5° × 0.5° POPE inventory v2.0 (Simon et al., 2024) and has been prepared as emissions for the chemistry‑transport model ICON‑ART PRIEST V1.0. Processing: Temporal interpolation: Annual total emission ratios for every grid cell and substance were linearly interpolated to monthly values, considering yearly totals are exactly conserved. Horizontal remapping: Conservatively remapped using cdo "remapcon" from the native 0.5° squared grid to the ICON R3B4 icosahedral grid used in ICON-ART PRIEST. Precursor species derivation: Two precursor species absent from the native POPE inventory; 8:2 fluorotelomer olefin (8:2 FTO) and 8:2 fluorotelomer iodide (8:2 FTI) are introduced following the split factors of Thackray et al. (2020 (48 % 8:2 FTOH, 48 % 8:2 FTO, 4 % 8:2 FTI). How to citePlease cite both the original POPE release and this derivative dataset: Simon, P. (2024). POPE model and Data v2.0. Zenodo. https://doi.org/10.5281/zenodo.12783504 Meza-Landero, H. A., Simon, P. (2025). POPE monthly emissions for ICON-ART PRIEST v1.0. Zenodo (https://doi.org/10.5281/zenodo.16539566) Reference to the original methods paper is also encouraged: Simon, P., Ramacher, M. O. P., Hagemann, S., Matthias, V., Joerss, H., and Bieser, J.: POPE: a Global Gridded Emission Inventory for PFAS 1950–2020, Earth Syst. Sci. Data Discuss. [preprint], https://doi.org/10.5194/essd-2024-236, in review, 2024. References: Simon, P. (2024). POPE model and Data v2.0. Zenodo. https://doi.org/10.5281/zenodo.12783504 Simon, P., Ramacher, M. O. P., Hagemann, S., Matthias, V., Joerss, H., and Bieser, J.: POPE: a Global Gridded Emission Inventory for PFAS 1950–2020, Earth Syst. Sci. Data Discuss. [preprint], https://doi.org/10.5194/essd-2024-236, in review, 2024. Thackray, C. P., Selin, N. E., & Young, C. J. (2020). A global atmospheric chemistry model for the fate and transport of PFCAs and their precursors. Environmental Science: Processes and Impacts, 22(2), 285–293. https://doi.org/10.1039/c9em00326f



