NO2– Activation and Reduction to NO by a Nonheme Fe(NO2)2 Complex
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https://figshare.com/articles/dataset/NO_sub_2_sub_sup_sup_Activation_and_Reduction_to_NO_by_a_Nonheme_Fe_NO_sub_2_sub_sub_2_sub_Complex/2271574
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The selective reduction of nitrite (NO2–) to nitric oxide (NO) is a fundamentally important chemical transformation related to environmental remediation of NOx and mammalian blood flow. We report the synthesis and characterization of two nonheme Fe complexes, [Fe(LN4Im)(MeCN)2](BF4)2 (1MeCN) and [Fe(LN4Im)(NO2)2] (2), geared toward understanding the NO2– to NO conversion. Complex 2 represents the first structurally characterized FeII complex with two axial NO2– ligands that functions as a nitrite reduction catalyst.
创建时间：
2016-02-17
