Synthesis and Characterization of a Stable High-Valent Cobalt Carbene Complex
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The formally CoIV carbene Co(OR)2(CPh2) is formed upon the reaction of diphenyldiazomethane with the cobalt bis(alkoxide) precursor Co(OR)2(THF)2. Structural, spectroscopic, and theoretical studies demonstrate that Co(OR)2(CPh2) has significant high-valent CoIVCPh2 character with non-negligible spin density on the carbene moiety.
创建时间：
2016-04-29
