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Redox-Dependent Franck–Condon Blockade and Avalanche Transport in a Graphene–Fullerene Single-Molecule Transistor

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https://figshare.com/articles/dataset/Redox_Dependent_Franck_Condon_Blockade_and_Avalanche_Transport_in_a_Graphene_Fullerene_Single_Molecule_Transistor/2089390
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资源简介:
We report transport measurements on a graphene–fullerene single-molecule transistor. The device architecture where a functionalized C60 binds to graphene nanoelectrodes results in strong electron–vibron coupling and weak vibron relaxation. Using a combined approach of transport spectroscopy, Raman spectroscopy, and DFT calculations, we demonstrate center-of-mass oscillations, redox-dependent Franck–Condon blockade, and a transport regime characterized by avalanche tunnelling in a single-molecule transistor.
创建时间:
2016-02-12
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