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Owing to the increasingly complex economic environment and difficult employment situation, a large number of new occupations have emerged in China, leading to job diversification. Currently, the overall development status of new occupations in China and the structural characteristics of new occupation practitioners in different cities are still unclear. This study first constructed a development index system for new occupation practitioners from five dimensions (group size, cultural appreciation, salary level, occupation perception, and environmental perception). Relevant data to compare and analyze the development status of new occupation practitioners were derived from the big data mining of China’s mainstream recruitment platforms and the questionnaire survey of new professional practitioners which from four first-tier cities and 15 new first-tier cities in China. The results show that the development level of new occupation practitioners in the four first-tier cities is the highest, and the two new first-tier cities, Chengdu and Hangzhou, have outstanding performance. The cities with the best development level of new occupation practitioners in Eastern, Central, and Western China are Shanghai, Wuhan, and Chengdu, respectively. Most new occupation practitioners in China are confident about the future of their careers. However, more than half of the 19 cities are uncoordinated in the five dimensions of the development of new occupation practitioners, especially those cities with middle development levels. A good policy environment and social environment have not yet been formulated to ensure the sustainable development of new occupation practitioners. Finally, we proposed the following countermeasures and suggestions: (1) Establish a classified database of new occupation talents. (2) Implement a talent industry agglomeration strategy. (3) Pay attention to the coordinated development of new occupation practitioners in cities.