Epoxidation of Bromoallenes Connects Red Algae Metabolites by an Intersecting Bromoallene Oxide - Favorskii Manifold
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DMDO epoxidation of bromoallenes gives directly a,b-unsaturated carboxylic acids under the reaction conditions. Calculated (wB97XD/6-311G(d,p)/SCRF=acetone) potential energy surfaces and 2H- and 13C-labeling experiments are consistent with bromoallene oxide intermediates which spontaneously rearrange via a bromocyclopropanone in an intersecting bromoallene oxide – Favorskii manifold.
创建时间：
2013-09-02
