Enantioselective Acylation of Silyl Ketene Acetals through Fluoride Anion-Binding Catalysis
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A highly enantioselective acylation of silyl ketene acetals with acyl fluorides has been developed to generate useful α,α-disubstituted butyrolactone products. This transformation is promoted by a new thiourea catalyst and 4-pyrrolidinopyridine and represents the first example of enantioselective thiourea anion-binding catalysis with fluoride.
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2011-09-07
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