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Switching of chiral phonons in ferroelectrics

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ESRF Portal2028-01-01 更新2026-04-23 收录
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https://doi.esrf.fr/10.15151/ESRF-ES-2166894199
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Chirality is one of the major topics in recent condensed matter physics due to chirality-induced functionalities and topological textures relating to symmetry breaking, e.g., in van der Waals materials. Driving a chiral mode can be a unique approach to manipulating ultrafast emergent phenomena and corresponding dynamics. Recently, our group successfully observed chiral phonons in chiral crystals of α-quartz using circularly polarized RIXS [Nature 618, 946 (2023)]. In principle, chiral phonons exist in other non-centrosymmetric crystals, such as polar (ferroelectric) materials, which we recently observed for a non-chiral but polar crystal LiNbO3. This result suggests that we can manipulate phonon chirality by flipping the polarization. We plan to demonstrate in situ electric field switching on free-standing (FS) films of BaTiO3 (BTO) using circularly polarized RIXS at the oxygen K-edge. Our results will open the possibility of manipulating phonon chirality and associated phonon angular
提供机构:
Paul Scherrer Institut, , 5232 , Villigen, SWITZERLAND; Paul Scherrer Institute, Photon Science, Forschungsstrasse 111, 5232, Villigen, CH; Paul Scherrer Institute, Center for Photon Science, Forschungsstrasse 111, 5232, Villigen psi, CH; Paul Scherrer Institute, Center for Photon Science, Forschungsstrasse 111, 5232, Villigen psi, SWITZERLAND
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2028-01-01
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