Global atmospheric particle formation from CERN CLOUD measurements: nucleation rate dataset
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Data S1 for paper "Dunne et al, (the CLOUD collaboration), Global atmospheric particle formation from CERN CLOUD measurements, Science 354 6316 (2016). Data contains nucleation rates and chamber conditions (including precursor gas concentrations) for inorganic binary and ternary (H2SO4-H2O) and (H2SO4-NH3-H2O) neutral and ion-induced nucleation measurements presented in the paper. These data were originally attached as supplemental to the paper, but are not currently available on the Science website (as of October 2024). Relative humidity units are percent. Care is needed to interpret all the data, for example not all ammonia values quoted were measured directly, some are inferred. See the supplementary materials of the paper for more discussion, and users of data at relative humidity other than (38+/-5)% are advised to discuss with the contact author Hamish Gordon. Ion production rate and nucleation rate units are per cm3 per second. The sulfuric acid units can be interpreted by noting that the value of 632 in the first data entry is 6.32x10^8 cm-3. Please cite the original Science article if you use these data: https://www.science.org/doi/10.1126/science.aaf2649
本数据集为论文《Dunne等人(CLOUD合作组):基于CERN CLOUD实验的全球大气粒子形成》(发表于*Science* 354卷第6316期,2016年)的补充数据S1。数据集包含论文中呈现的无机二元(H₂SO₄-H₂O)及三元(H₂SO₄-NH₃-H₂O)体系的中性成核与离子诱导成核的成核速率及实验舱条件(含前驱体气体浓度)。该数据最初作为论文补充材料附带,但截至2024年10月,Science官方网站已无法获取该数据集。 相对湿度单位为百分比。解读所有数据时需谨慎:例如,并非所有引用的氨气浓度均为直接测量所得,部分为推算值。详细说明请参见论文的补充材料;若使用者需使用相对湿度不为(38±5)%的数据,建议与通讯作者Hamish Gordon联系。离子产生速率与成核速率的单位为每秒每立方厘米。硫酸浓度的单位可通过如下方式理解:首个数据条目中的数值632实际代表6.32×10⁸ cm⁻³。 若使用本数据集,请引用该原始*Science*论文:https://www.science.org/doi/10.1126/science.aaf2649



