合成气提质与吸附强化一体化制氢关键技术数据集

于2020年1月至2022年12月在太原理工大学省部共建煤基能源清洁高效利用国家重点实验室完成相关工作。实验数据来自固定床制氢反应装置及热重分析仪（STA449F5）；X-射线衍射仪（Rigaku D/Max-3B）；扫描电子显微镜（JEOL-TM3000）、化学吸附仪（Autochem II2920）、物理吸附仪（Quantachrome iQ Autosorb-1）等相关表征仪器。通过选用不同前驱体类型及比例制备尖晶石结构复合催化剂，在不同焙烧温度处理后，经700 °C还原1 h复合催化剂；采用自制固定床反应器完成制氢性能评价，产气组成由气相色谱仪进行检测。绘图软件是Origin。

This work was conducted at the State Key Laboratory of Clean and Efficient Utilization of Coal-based Energy, Taiyuan University of Technology (jointly constructed by the provincial and ministerial authorities), from January 2020 to December 2022. Experimental data were collected from a fixed-bed hydrogen production reactor, a thermogravimetric analyzer (STA449F5), an X-ray diffractometer (Rigaku D/Max-3B), a scanning electron microscope (JEOL-TM3000), a chemical adsorption analyzer (Autochem II2920), a physical adsorption analyzer (Quantachrome iQ Autosorb-1), and other related characterization instruments. Spinel-structured composite catalysts were prepared by adopting precursors with different types and ratios. After being calcined at various temperatures, the catalysts were reduced at 700 °C for 1 hour. Hydrogen production performance evaluation was performed using a self-made fixed-bed reactor, and the composition of the product gas was detected by gas chromatography. Origin was utilized for plotting the figures.